Extensive progress has recently been made in our understanding of heavy-element production via the r-process in the universe, specifically with the first observed neutron star binary merger (NSBM) event associated with the gravitational-wave signal detected by LIGO, GW170817. The chemical abundance patterns of metal-poor r-process-enhanced stars provide key evidence for the dominant site(s) of the r-process and whether NSBMs are sufficiently frequent or prolific r-process sources to be responsible for the majority of r-process material in the universe. We present atmospheric stellar parameters (using a nonlocal thermodynamic equilibrium analysis) and abundances from a detailed analysis of 141 metal-poor stars carried out as part of the R-Process Alliance (RPA) effort. We obtained high-resolution "snapshot" spectroscopy of the stars using the MIKE spectrograph on the 6.5m Magellan Clay telescope at Las Campanas Observatory in Chile. We find 10 new highly enhanced r-II (with [Eu/Fe]>+1.0), 62 new moderately enhanced r-I (+0.3<[Eu/Fe]<~+1.0), and 17 new limited-r ([Eu/Fe]<+0.3) stars. Among those, we find 17 new carbon-enhanced metal-poor (CEMP) stars, of which five are CEMP-no. We also identify one new s-process-enhanced ([Ba/Eu]>+0.5) and five new r/s (0.0<[Ba/Eu]<+0.5) stars. In the process, we discover a new ultra-metal-poor (UMP) star at [Fe/H]=-4.02. One of the r-II stars shows a deficit in {alpha} and Fe-peak elements, typical of dwarf galaxy stars. Our search for r-process-enhanced stars by RPA efforts has already roughly doubled the known r-process sample.