Optical (BVRI) photometric measurements of a sample of 564 candidate cool subdwarfs in the nearby halo are presented. The stars generally span the color range 0.4<(B-V)<1.8; hence, the sample is composed of early F- through early M-type stars on the subdwarf sequence. The sample is selected from the revised NLTT catalog of Gould and Salim and Salim and Gould via a reduced proper motion diagram. The photometry is precise and accurate; in particular, for stars with 9<V<13.5 the photometry is accurate to 0.013, 0.015, 0.012, and 0.013mag in V, B-V, V-R, and V-I, respectively. For stars with 13.5<V<16 the photometry is accurate to 0.022, 0.018, 0.013, and 0.018mag in the same bands.